03 - Ionization chambers Jaroslav Adam Czech Technical University in Prague Version 1.0 Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 1 / 132 Principle of operation Charged particle getting through a volume of a gas or noble liquid Interaction proceed through ionization and end excitation of the molecules, electron-ion pairs are created Ion can be created directly by the incident particle, or by the δ-electrons, when the energy from the primary particle if first transferred to the electron which acquires enough energy to make further ionization Electric field is applied by the electrodes, electrons and ions drift to them If the field is high enough, drifting electrons can also ionize the gas (proportional counters) After further increase of the field strength, electrons emit UV light on the anode (Geiger-Muller counter) Electronic signal at the output, pulsed or current regime Position sensitivity by segmenting one of the electrodes (xy ) and by timing measurement (z) Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 2 / 132 Ionization detectors without amplification Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 3 / 132 Number of ion pairs Minimum energy W to be transferred from the incident particle to create at least one ion pair Quantified as average energy loss to create the pair Given by the least tightly bound shell, W = 10 - 25 eV Non-ionizing energy loss (excitation) makes number of pairs lower Fully stopped 1 MeV particle produces 30 000 ion pairs Number of pairs is important for resolution Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 4 / 132 Fano factor Fluctuation in number of pairs affect the energy resolution The simplest approach postulate Poisson statistics for number of ion pairs (σ = √ N) Fano factor makes correction to predicted variance to get observed variance Fano factor = 0 if all incident energy converted into pairs, no statistical fluctuation In gases Fano factor < 1, Poisson distribution valid but fluctuations are smaller than √ N Significant in pulse mode Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 5 / 132 Principle of ionization chamber Figure : Planar ionization chamber Suppose two metallic electrodes at distance D covering volume of a gas or noble liquid Voltage V applied to anode (thousands of kV) Number of electrons n− given by the number of minimum-ionizing-particles (mip) n− = n dE Dρ W dx (1) ρ is the density and dE/dx is energy loss per g cm−2 Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 6 / 132 Charge carriers in gas/liquid volume Several processes applies to the ion pairs Drift movement by external electric field Diffusion due to random thermal movement Charge transfer Recombination Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 7 / 132 Drift movement Electrostatic force moves the charges, positive ions opposite to electrons and negative ions Drift of electrons characterized by drift velocity in electric field E = V /D vd (e) = dx µe V µe = E= dt p pD (2) Electron mobility µe given in unit of bar cm2 V−1 s−1 , p is the gas pressure Mobility of ions is about 1000 less than of electrons Description with mobility provides calculation of readout times ms for ions, µs for electrons Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 8 / 132 Saturation of the drift velocity Figure : Electron velocity vs. filed No increase in drift velocity after reaching it’s maximum, only in some gases Hydrocarbons, argon-hydrocarbon mixtures In non-saturation gases, E/p proportionality holds up to high fields Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 9 / 132 Diffusion Thermal movement with mean free path of about 10−6 - 10−8 m More important for electrons since their thermal velocity is bigger Point-like collection of electrons form Gaussian spatial distribution widening with time Widening in one direction x, y or z given by diffusion coefficient D √ σ= 2Dt (3) D is given by kinetic gas theory or the process is described by a transport model Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 10 / 132 Charge transfer collisions Electron transfer from neutral gas molecule to positive ion in mutual collision Significant in mixtures, net positive charge transfered to species with lowest ionization energy Negative ion can be formed by capturing of free electron (oxygen) Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 11 / 132 Recombination Free electron captured by positive ion making ordinary neutral atom Positive and negative ions recombine, most probable compared to electron and ion case Original charge is lost, no contribution to final signal Recombination rate given by density of positive and negative species n+ and n− and recombination coefficient α dn+ dn− = = −αn+ n− dt dt Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers (4) Version 1.0 12 / 132 Initial recombination Recombination of electron with it’s parent ion Mainly for heavy ionizing particles (low energy α), minimal for mip Independent of the event rate Suppressed by applying electric field larger than Coulomb field of electron-ion system Quantified as a ratio of charge after initial recombination Qrec to the amount of initial charge Q0 (Onsager 1938) " rkT Qrec = exp − 1+E Q0 r0 e3 2k 2 T 2 !# (5) rkT = e2 /kT is Onsager length or radius, r0 is thermalization length, k is the Boltzmann constant, T is temperature, E is applied electric field, is electric permitivity of the medium Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 13 / 132 Columnar recombination Electron-ion pairs created in column along particle trajectory Recombination may occur with neighboring ion when electrons are drifting in electric field Depends on the angle between incident particle and electric field Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 14 / 132 Volume recombination Recombination during drift towards electrodes Unlike initial/columnar recombination, this depends on irradiation rate Suppressed by fast charge separation and collection -> high electric field Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 15 / 132 Carrier density evolution under drift and diffusion Initial Gaussian distribution of electrons n− and ions n+ along z in column of radius b n± (t = 0) = N0 exp πb2 − x2 + y2 b2 ! (6) Evolution in time is given by dn± ∂n± = ∓µ± E sin φ + D± ∆n± − kr n− n+ dt ∂x (7) D± = µ± kT /e, φ is emission angle vs. field, kr is columnar recombination factor Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 16 / 132 Ionization current, DC ion chamber Constant irradiation rate creates constant formation of ion pairs Steady-state current is measure of the rate Supposing negligible recombination and efficient charge collection Figure : Planar ionization chamber Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 17 / 132 Current-voltage characteristics Electric field by external voltage Current in the circuit equal to ionization current at equilibrium Increasing voltage begins to separate the charges that would recombine High electric field makes recombination negligible After ion saturation, all charges are collected, on increase in current when increasing the voltage Standard operation of ion chambers, current in the circuit is an indication of the rate of ion pairs formation Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 18 / 132 Saturation current Recombination, especially columnar recombination require high voltage Volume recombination important at high irradiation intensity Higher voltage required to get true saturation current More important in neutron measurement, where heavy fragments are detected With chambers filled by ambient air, recombination depends on humidity Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 19 / 132 Perturbations in current due to diffusion Imbalance in steady-state situation supposing uniform production of ions within the chamber Larger concentration of positive ions close to cathode, opposite for electrons close to anode Gradient in concentration formed, diffusion opposite to drift Perturbation in measured current in planar chamber given by − ∆I kT = I eV (8) is ratio of average energy of charge carrier, kT /e ≈ 2.5 × 10−2 V at room temperature close to one for ions, but several hundreds for electrons Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 20 / 132 Losses of saturation current due to diffusion close to one for ions, but much larger, several hundreds for electrons Minimized by high voltage Columnar recombination not fully eliminated Separate measurements of ionization current as a function of voltage 1/I as a function of 1/V to determine true saturation current Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 21 / 132 Operation of DC ion chamber No special requirement on gas since negative charge can be collected as free electrons as well as negative ions Only recombination could affect the amount of charge, suppressed by high enough voltage Few centimeters and tens of hundreds of volts sufficient to reach saturation Air for gamma-ray exposure, denser gases like Argon to increase ionization density Pressure about 1 atmosphere, higher to increase sensitivity Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 22 / 132 Geometry of ionization chamber Electric field given by geometry of electrodes Uniform electric field with planar geometry Cylindrical geometry with electrical field as E(r ) = U0 r ln(ra /ri ) Figure : Cylindrical ionization chamber Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 23 / 132 Insulators Small values of ionization current, < 10−12 A Resistance of insulator at least 1016 Ω to keep leakage current below 1% for U = 100 V Leakage by moisture absorbed on surface suppressed by the guard rings and smooth surface of insulators Plastics or ceramic for higher irradiation Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 24 / 132 Measurement of gamma-ray exposure with ion chambers Amount of charge in air-filled ionization chamber Charge is measure of exposure, ionization current gives exposure rate Requires to measure ionization of all secondary electrons, mean free pairs several meters compensation for secondary electrons needed Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 25 / 132 Compensation by free-air ionization chamber Collimated X-rays, compensation in horizontal direction Compensation of electrons escaping the sensitive volume by electrons emerging elsewhere Up to gamma-ray of 100 keV Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 26 / 132 Air equivalent compensation Reduces space requirements for higher gamma-rays energies, wall thickness less than 1 cm Exposure rate given by saturation current Is and mass M in active volume R= Jaroslav Adam (CTU, Prague) Is M DPD_03, Ionization chambers (9) Version 1.0 27 / 132 Absorbed dose Based on average energy loss per ion pair W (joule / ion pair), relative mass stopping power Sm and number of ion pairs per unit mass (ion pairs per kg) Dm = W · Sm · P (10) Dm is then in grays (J kg−1 ) Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 28 / 132 DC chambers for radiation survey Radiation monitoring Saturation current in closed volume of several cm3 Dose measured by charge integration Initial charge on the chamber, drop in voltage measures total integrated ionization charge Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 29 / 132 Ionization dosimeter Cylindrical air capacitor, initially charged at some voltage V0 Discharged by the radiation Voltage reduction measures absorbed dose Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 30 / 132 Calibration of radiation source Saturation current depends only on geometry, long time stability Current from unknown source compared with standard under same geometry Chambers with thousands of cm3 Pressured gas for higher sensitivity Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 31 / 132 Geometry for calibration of gamma-ray sources Calibration for gamma-ray sources, ionization current for small displacement of the source Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 32 / 132 Measurement of radioactive gases Radioactive gas as constituent of fill gas, sampled as continuous flow ¯ and total Ionization current I given by average energy deposition per gas disintegration E activity α I= ¯ Eαe W (11) Principle of smoke detectors where ionization current from internal alpha source decreases due to presence of the smoke in sampled air Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 33 / 132 Remote sensing of ionization Positive and negative ions in the air survive for minutes before recombination Flow of air is transported to a chamber outside the source of radiation LRAD - Long Range Alpha Detector: Sample of alpha-contaminated material in container, air flowing though it Positive and negative ions carried into an ion chamber Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 34 / 132 Pulse mode operation Each radiation quantum provides with distinguishable signal pulse Application in radiation spectroscopy Alpha spectrometry Neutron detection Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 35 / 132 Equivalent circuit of ion chamber Chamber presented by it’s capacity C Voltage V0 on load rezistor R Drifting charges from ionization create induced charge on electrodes Voltage drops from equilibrium V0 , giving output pulse VR Slow return to equilibrium according time constant RC If RC > time to collect all charges, amplitude of the pulse measures the original charge Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 36 / 132 Equivalent circuit of ion chamber The ion chamber behaves as parallel connection of resistor and capacity, called RC circuit Time dependence of voltage V given by capacity C and resistivity R C dV V =I= dt R (12) Response to initial charge giving voltage V0 is V (t) = V0 e−t/RC Jaroslav Adam (CTU, Prague) (13) DPD_03, Ionization chambers Version 1.0 37 / 132 Electron sensitive mode Time to collect electrons ∼ µs, time for ions ∼ ms Collection of all charges would require RC of orders of >ms This would mean low pulse rate only and interference from microphonic signals For electron sensitivity, RC between electron and ion collection time Negative ions no longer allowed Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 38 / 132 Pulse shape in planar chamber Constant electric field E = V /d Uniform equipotentials parallel to electrode surfaces Ions supposed to be formed at equal distance x where electric potential is Ex Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 39 / 132 Pulse shape of electron and ion collection Derivation of VR (t) based on energy conservation RC long enough to collect all charges Energy in capacitance 1/2CV02 is energy source to move the charges Drift velocity v − for electrons and v + for ions, n0 is number of ion pairs 1 1 2 CV02 = n0 eEv + t + n0 eEv − t + CVch 2 2 Vch V0 V0 + Vch ' 2V0 and ' d d VR = (14) (15) n0 e + (v + v − )t dC (16) After collecting the electrons (time t − ≡ x/v − ) VR = Jaroslav Adam (CTU, Prague) n0 e + (v )t dC DPD_03, Ionization chambers (17) Version 1.0 40 / 132 Pulse shape of electron and ion collection After collecting the ions (time t + ≡ (d − x)/v + ) n0 e [(d − x) + x] dC n0 e VR = C (18) VR = (19) If RC t + , maximum amplitude of the pulse is Vmax = n0 e C (20) Independent of position of incident ionization Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 41 / 132 Pulse shape of electron and ion collection Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 42 / 132 Pulse shape in electron sensitive operation Pulse shape given by electrons Amplitude sensitive to position of incident radiation V |elec = n0 e x · C d (21) Monoenergetic radiation produces a range of pulses Removed by dividing the ion chamber by adding a grid Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 43 / 132 Gridded ion chamber Designed to remove amplitude position dependency All interactions between the grid (Frisch grid) and the cathode Grid at intermediate potential and transparent for electrons Grid-anode voltage drops after electrons pass through the grid Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 44 / 132 Electron signal in gridded ion chamber Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 45 / 132 Electron signal in gridded ion chamber With RC larger than electron collection time and grid-anode spacing d, signal on load resistor is VR = n0 e − v t dC (22) Maximum voltage is Vmax = n0 e C (23) Allows to operate at short RC Pulse independent of position of incident radiation But signals of order of < 10−5 V Can not be measured directly, amplification needed Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 46 / 132 Statistical limit to energy resolution Number of charges n0 and fano factor F gives statistical limit Supposing fully stopped α at energy E = 5.5 MeV in gas with W = 30 eV/ion pair and F = 0.15 n0 = Ed = 1.83 × 105 ion pairs W (24) Standard deviation as square root of variance σn0 = Jaroslav Adam (CTU, Prague) p Fn0 = 166 DPD_03, Ionization chambers (25) Version 1.0 47 / 132 Statistical limit to energy resolution FWHM of Gaussian distribution for n0 and particle energy FWHM(n0 ) = 2.35σn0 = 390 (26) FWHM(E) = 2.35σn0 · W = 11.7 keV (27) Relative energy resolution to the deposited energy R= 2.35σn0 W = 0.123% Ed (28) Good theoretical resolution can not be achieved due to electronic noise Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 48 / 132 Charged particle spectroscopy with pulse-type ion chamber Some advantages vs. semiconductor or scintillator detectors Arbitrary size and geometry Gas dielectric cable 3500 m long was used as a beam-loss monitor at SLAC Gas pressure to adjust stopping power or effective thickness Radiation resistant, simple design Low level alpha particles, cross sectional area 500 cm2 Bragg curve spectroscopy: analysis of pulse shape from incident particle parallel to the field, can distinguish particle species Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 49 / 132 Alpha spectroscopy with ionization chamber Fisch grid ionization chamber filled by argon allows to separate two uranium isotopes Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 50 / 132 Measurement of purity of liquid argon by ionization chamber α-cell ionization chamber used by ATLAS to monitor liquid argon fill of electromagnetic calorimeters Electron charge from α ionization Detection of impurities in argon Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 51 / 132 Proportional counters Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 52 / 132 Charge multiplication in the gas Late 1940s, effect of gas multiplication More ion pairs compared to ionization chamber Low energy X-rays Neutron detection Pulse mode most common operation Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 53 / 132 Avalanche formation Kinetic energy of the electron sufficient to make secondary ionization Field at least 106 V m−1 Gas multiplication: secondary electrons also ionize after acceleration Townsend avalanche dn = αdx n Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers (29) Version 1.0 54 / 132 Townsend coefficient vs. field Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 55 / 132 Regions of operation Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 56 / 132 Cylindrical geometry Field with anode wire radius a, cathode inner radius b and applied voltage V is E(r ) = Jaroslav Adam (CTU, Prague) V r ln(b/a) DPD_03, Ionization chambers (30) Version 1.0 57 / 132 Field as a function of radius Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 58 / 132 Avalanche from a single electron, MC transport model Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 59 / 132 Construction design Figure : Cross sectional view, dimensions in cm Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 60 / 132 2π proportional counter Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 61 / 132 4π proportional counter Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 62 / 132 Fill gas Gases without significant electron attachment Oxygen or electronegative impurities must be removed in flow-counters Sealed counters more convenient to use, but may have limited lifetime Polyatomic gas (methane) to prevent photon-induced effects, component called quench gas Most common proportional gas is 90% argon + 10% methane (P-10 gas) Penning effect - component with ionization energy lower than excitation energy of principal gas Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 63 / 132 Gas multiplication factor Single electron response by avalanche created by one electron outside multiplication region Total charge by n0 original pairs with gas multiplication factor M is Q = n0 eM Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers (31) Version 1.0 64 / 132 Gas multiplication factor vs. voltage Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 65 / 132 Space charge effects Reduction of the field near anode due to positive ions Self induced effects resulting from high gas gain, does not depend on pulse rate General space charge effect is cumulative for different avalanches, also for lower gain M should just satisfy signal-to-noise requirement to prevent space charge effects Simple check by varying the voltage and looking for suppression of large pulse amplitudes Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 66 / 132 Energy resolution Fluctuations in n0 and in multiplication Variance of pulse amplitude given by ion pair fluctuation and single-electron multiplication variations Furry distribution of number of electrons in a given avalanche, probability of ionization depends only on E Polya distribution for higher fields, ionization depends on electron’s history, not only on E Distribution of pulse amplitude approaches Gaussian for large n0 (more than 20) Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 67 / 132 Energy resolution Fractional standard deviation of the peak (FWHM/2.35), P-10 gas at 1 atm pressure Open circles: standard tungsten anode Full circles: improved uniformity Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 68 / 132 Systematic variations in gas multiplication factor Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 69 / 132 Time characteristics of the signal pulse Output pulse is sum of drift time of free electrons to reach multiplication region and multiplication time required for the avanlache Drift time greater than multiplication time Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 70 / 132 Equivalent circuit of proportional counter seen by developing signal Derivation of pulse shape utilizes energy conservation of charge moving across the capacitor Most of the pulse amplitude from positive ion drift Collection time of all ions long, hundreds ms, but large fraction of signal developed early of ion drift, fraction of µs Spread in electron drift times (ionizations along radius) makes spread in rise time of output pulse Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 71 / 132 Shape of output pulse Solid curve represents initial ionization at fixed radius (constant drift time) Dashed line is for uniform ionization along the radius Rise time minimized by high electric field in drift region and gases with high electron drift velocity Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 72 / 132 Electron drift velocity Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 73 / 132 Variations of pulse rise time Pulse shaping with short time constant removes slow component of rise time Amplitude less than of full collection, effect of balistic deficit Shape of pulse would vary with radial position of original ion pairs Minimized by shaping time larger than variation in rise time Can be used to separate signal α events from electron background Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 74 / 132 Spurious pulses Satellite afterpulses from secondary processes following desired signal Removed by amplitude discrimination since correspond to single-electron avalanche Effect increases with high value of gas multiplication Optical photons by excited atoms within the avalanche, low energy electron at cathode surface through photoeffect Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 75 / 132 Operating voltage Signal pulse for every particle with enough energy deposit Sensitivity to more than one avalanche to suppress space charge effects and spurious pulses Lower values of multiplication factor, some number of original ion pairs to create detectable signal Counting curve to select appropriate operating voltage (counting rate vs. voltage at same source condition), looking for flat region Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 76 / 132 Alpha counting Monoenergetic charged particles of range less than dimensions of the chamber Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 77 / 132 Beta counting Range greater than chamber dimensions, smaller pulses compared to alpha 4π counter for absolute beta activity Greater range advantage for mechanical source backing Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 78 / 132 Mixed alpha and beta sources Two readout channels for alpha and beta Separation by amplitude Background from cosmic rays or ambient gamma (most sources) does not affect alpha window Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 79 / 132 X-ray and gamma-ray sources Fraction of incident photons absorbed in 5.08 cm of proportional gases at 1 atm pressure Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 80 / 132 X-ray and gamma-ray sources X-ray spectroscopy by full absorption of photoelectrons, full energy peaks in pulse spectrum Small signal enhanced by internal gas multiplication Gamma rays in Geiger-Muller region Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 81 / 132 Response function for low-energy X-rays Characteristic X-rays after photoabsorption of primary radiation may escape without interaction Suppressed with K-shell energy above incident X-ray energy Requirements to entrance window, beryllium or aluminum 50 - 250 µm Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 82 / 132 Fluorescence gating Electronic separation of photoelectric absorption of incident photon and absorption of consequent characteristic X-ray Proportional counter as series of independent cells, X-ray absorbed in different cell Two pulses in time coincidence corresponding to full absorption, escape peak avoided Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 83 / 132 Tissue equivalent proportional counter Dosimetry of gamma rays and neutrons Walls and gas mixture mimic elemental composition of biological tissue Steady flux of secondary particles from the wall Determines quality factor for equivalent dose Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 84 / 132 Parallel plate avalanche counters Heavy charged particles which would impose radiation damage to solid state detectors Parallel plate electrodes, proportional gas at low pressure Particle species separation by specific energy loss For gap of 1 mm, fast component from electrons in ns with high field, time resolution 160 ps Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 85 / 132 Position-sensitive proportional counters Avalanche occurs around small portion of anode wire length Position of avalanche is indicator of axial position in cylindrical geometry Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 86 / 132 Charge division method Anode with significant resistance per unit length Two amplifiers at the ends, sum related to conventional pulse, proportion to the position of the interaction Alternatively relative rise time could be analyzed, longer rise time for pulse far from amplifier Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 87 / 132 Multiwire proportional counters (MWPC) Field by equidistant grid of anode wires between two parallel cathode plates High field region only in immediate vicinity of the anodes Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 88 / 132 Two-dimensional MWPC Cathodes divided into perpendicular strips Centroid of discharge located by center-of-gravity technique Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 89 / 132 Multicell proportional counter Cylindrical independent cells Coincidence measurement for process selection or background rejection Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 90 / 132 Gas proportional scintillation (GPS) counters Signal pulse from visible or UV photon emitted by excited gas atoms or molecules Excited in inelastic collisions between drifting electrons and neutral atoms Photons detected by photomultiplier or silicon avalanche photodiodes Greater light yield compared to conventional scintillator Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 91 / 132 GPS with uniform field Avoids recombinations in low-field region Time duration measures depth of the interaction Depth dependence canceled by dividing the total light yield by the time duration Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 92 / 132 Light properties in GPS Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 93 / 132 Voltage characteristics of GPS (1) charge gain, (2) light gain, (3) secondary light per collected electron Secondary light at much lower voltage than the onset of charge multiplication (3 kV here) Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 94 / 132 Microstrip gas chamber (MSGC) Narrow anode metallic strips (10 µm) on substrate Quick collection of ions, clearing the space charge Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 95 / 132 Two-dimensional MSGC Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 96 / 132 Gas electron multiplier (GEM) Preamplification in gas to allow lower voltage readout of microstrip detector GEM foil of insulating material, both surfaces covered by metallic cladding Hole density 50 per mm2 Holes of 140 µm pitch and 70 µm diameter Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 97 / 132 Electric field in GEM foil Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 98 / 132 Cascade of GEM foils Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 99 / 132 Micromegas (micro-mesh gaseous structure) Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 100 / 132 Resistive Plate Chamber (RPC) Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 101 / 132 Time Projection Chamber (TPC) of the ALICE experiment 3D position and dE/dx using volume of 90 m3 of Ne/CO2 /N2 (90/10/5) divided into two sectors of 2.5 m Voltage 100 kV on central electrode, drift field 400 V m−1 Electron drift velocity 2.7 cm µs−1 , maximum drift time 92 µs Readout by MWPC with cathode pad readout mounted in trapezoidal sectors at each end plate Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 102 / 132 MWPC readout of ALICE TPC Figure : Cross sectional view along the wires Figure : Cross sectional view perpendicular to the wires DPD_03, Ionizationwire chambers Grid of anode wires above pad plane, cathode plane and gating grid Jaroslav Adam (CTU, Prague) Version 1.0 103 / 132 MWPC readout of ALICE TPC Grid of anode wires above pad plane, cathode wire plane and gating grid Active area of 32.5 m2 Wire geometry and pad size dependent on radial track density Anode to cathode distance 2 and 3 mm, gain up to 20 000 560 000 readout pads of 4 × 7.5 mm2 for inner chambers and 6 × 10 mm2 and 6 × 15 mm2 in outer chambers Gate opens for electrons from the drift volume by the collision trigger (6.5 µs after the collision) for the duration of drift time, 92 µs, prevents the space charge of positive ions from drifting back from multiplication region Gating reduces drift of electrons by a factor more than 105 Position calibration by internal laser system, artificial straight tracks perpendicular to the beam axis, laser trigger rate up to 10 Hz Analog-to-digital (ADC) sampling with 6 ADC counts per fC Position resolution 1100 - 800 µm in r φ and 1250 - 1100 µm in z dE/dx resolution 5 % for isolated tracks, 6.8 % at high multiplicity Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 104 / 132 TPC laser calibration seen on run monitoring Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 105 / 132 Particle identification by dE/dx in TPC Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 106 / 132 Upgrade of TPC Expected rate 50 kHz of Pb-Pb, 5 interactions within maximal electron drift time, 10 events superimposed from past+future time window Untriggered readout without use of gating grid Readout by GEM foils instead of MWPC, field 50 kV/cm in the hole Suppression of back flowing ions One side segmented to reduce total charge on the foil, segments coupled by resistors Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 107 / 132 Simulation of GEM Light lines - electrons, dark lines - ions, spots - ionization occurence Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 108 / 132 Geiger-Mueller Counters Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 109 / 132 G-M counter Introduced in 1928, one of the oldest detectors Higher field than in proportional counter One avalanche can create at least one another avalanche, chain reaction All pulses have same amplitude, 109 - 1010 ion pairs Pulse amplitude in volts, no need for external amplification Counting rate limited by dead time Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 110 / 132 Geiger discharge Excited molecules of neutral gas in Townsend avalanche, together with positive ions They emit visible or UV light, may be absorbed by photoeffect at any place of the tube, new free electron created Or free electron created by absorption at cathode New avalanche from the free electron after reaching the multiplication region around anode Subcritical proportional tube: n00 p 1 with n00 number of excited molecules in typical avalanche and p the probability of photoabsorption Geiger discharge with single avalanche multiplication 106 - 100 has n00 bigger, criticality achieved as n00 p ≥ 1 Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 111 / 132 G-M region Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 112 / 132 Geiger discharge propagation New avalanches created close to the original one, new electrons have to reach anode region Spread of Geiger discharge along the anode wire with propagation velocity 2 − 4 cm µs−1 over entire length of anode, few µs after initiating event Avalanches at random positions around anode, electrons collected by anode, secondary positive ions around the multiplication region Field reduced by space charge of the ions, multiplication reduced, Geiger discharge terminated Amount of needed space charge independent of initial ionization, the reason for same pulse amplitude Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 113 / 132 Amplitude of Geiger discharge Amplitude increases with higher applied voltage More space charge needed to reduce the field below criticality Overvoltage defined as voltage above minimum required for Geiger discharge initiation Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 114 / 132 Fill gases Same requirements as for proportional counters since charge multiplication is needed (no negative ions...) Noble gases, helium, argon, quenching component n00 increases with E/p (electric field to gas pressure), G-M as sealed tube with pressure less than atmospheric Voltage 500 - 2000 V for anode of 0.1 mm diameter Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 115 / 132 Quenching Slow drift of positive ions after Geiger discharge termination to the cathode, neutralization with electron from cathode surface Energy needed = sum of gas ionization energy and energy to extract the electron from cathode (work function) If (gas ionization energy) = 2 × (work function), another free electron emerges from the cathode surface At least one free electron from cathode with large amount of positive ions Will drift towards anode to make new Geiger discharge Cycle would repeat, continues output of multiple pulses No problem for proportional counters, number of ions smaller, only spurious pulses Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 116 / 132 External quenching Needed any method to prevent excessive multiple pulsing Reduction of high applied voltage for some fixed time after the pulse below gas multiplication Time greater than transit of positive ions to the cathode (hundreds of ms) and transit time of free electron (few µs) Value of R selected high enough (108 Ω), so RC is of ms Several ms for anode to return to nominal operating voltage, low counting rate Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 117 / 132 Internal quenching Component of quench gas added to primary fill gas, concentration 5 - 10 % Smaller ionization potential, more complex molecular structure Multiple pulsing prevented by charge transfer collisions, positive charge of primary gas ion transfered to quench gas molecule, original ion neutralized before reaching cathode Ions of quench gas at cathode with some concentration of quench component At cathode, the excess energy dissociates the more complex molecule, emission of free electron suppressed, no additional avalanches Organic molecules, ethyl alcohol, ethyl formate Limit of 109 counts due to consumption of quench gas Problem avoided by halogens as quench gas (chorine, bromine), spontaneous recombination after dissociation Limit to lifetime then by contamination of reaction products from the discharge and polymer deposition on anode surface Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 118 / 132 Shape of the output pulse Signal of multiple avalanches from secondary electrons Spread in time for them to reach multiplication region Rise time of few µs Electric field distorted from the space charge of positive ions Fast rise and slow rise from ions drift, time constant less than 100 µs to eliminate slow component Loss in amplitude tolerated due to large amount of charge Delay in response by drift of original electrons to multiplying region, applies for timing with G-M as time uncertainty Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 119 / 132 Dead time Drift of positive ions outwards, recovery of filed in multiplying region After drift to some distance, the field permits new Geiger discharge, lower intensity in the beginning First pulses reduced in amplitude Full field and full amplitude after all ions neutralized at the cathode Dead time = time between initial pulse and second Geiger discharge, regardless of the magnitude, 50 - 100 µs Resolving time = time for pulse of amplitude high enough to be registered, dead time may include also recovery time in practical application Recovery time = time to return to the original state, pulse of full amplitude Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 120 / 132 Dead time behavior Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 121 / 132 Geiger counting plateau Dependence of measured counting rate on voltage with constant rate from radiation source Counter threshold Hd , no pulses if amplitude is below Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 122 / 132 Onset of continues discharge Corona discharge by irregularities on anode wire or quenching failure Decrease of voltage needed Operating voltage just sufficient for the flat region, reduces quench gas consumption Low amplitude tail causes some slope of the counting curve Hysteresis in counting curve due to charges on insulators Linearity of the plateau measures quality of G-M Organic quenched tubes have slope of 2 - 3 % with change in voltage by 100 V Halogen quenched tubes have greater slope, but larger lifetime and lower operating voltage Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 123 / 132 End-window Geiger tube Fine anode wire, less requirements on uniformity of the wire and of the electric field Cylindrical cathode of metal or glass with metallized inner surface Thin window for short-range particles, differential pressure More robust window for beta or gamma Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 124 / 132 Other design of Geiger tube Wire loop anode in cathode of arbitrary volume Needle counters - sharply pointed needle, field as 1/r 2 (1/r for cylindrical geometry), used for smaller active volume Source in counting volume for low-energy particles 14 C detection by gas mixture of CO2 with counter gas for high counting efficiency Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 125 / 132 Counting electronics R is load resistance for signal development Cs is capacitance of the tube and wiring, parallel with R RCs ∼ few µs for fast-rising component Coupling capacitor Cc to block high voltage on the tube, only signal pulse transmitted, RCc larger than pulse duration Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 126 / 132 Counting efficiency for charged particles 100 % for any charged particle entering the active volume since a single ion pair triggers full Geiger discharge Effective efficiency given by the window of the tube, absorption or backscattering For alpha counting window with 1.5 mg/cm2 Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 127 / 132 Efficiency for neutrons Rare application for neutron detection Low capture cross section for Geiger gases Gamma-ray discrimination not possible, all pulses have same size Neutron-induced reactions detected by proportional counters, large amplitude from such reactions Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 128 / 132 Counting efficiency for gamma rays Interaction in solid wall of the counter, secondary electron needs just to emerge into active volume 1 - 2 mm of innermost layer of the wall Efficiency increased with high-Z material of the cathode (bismuth Z = 83) Low-energy gamma may interact with fill gas, xenon and krypton (high-Z) enhance the efficiency up to 100 % for photon energies 10 keV Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 129 / 132 Counting efficiency for gamma rays Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 130 / 132 Dead time correction by time-to-first-count method Losses by dead time significant at rates of few hundred counts per second Method based on switching two voltages on the tube After Geiger discharge, voltage set below value for multiplication for time longer than recovery at reduced voltage, 1 - 2 ms (waiting time) Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 131 / 132 Dead time correction by time-to-first-count method Series of measurements of time from end of waiting time and next true event Average of these intervals equals to 1/r with r the true event rate Voltage switching should be fast for reasonable timing accuracy, tens of µs Counting rate extended up to 105 counts per second Statistical uncertainty given by number of measured time intervals At least 104 time intervals for 1 % statistical accuracy Jaroslav Adam (CTU, Prague) DPD_03, Ionization chambers Version 1.0 132 / 132
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